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Schematic top and side views of (a) a supercell of the MoS2 monolayer including 90 atoms in the absence of the gas molecule and in the presence of the (b) CO, (c) CO 2 and (d) NO adsorbates. Graphene-Based Chemical Vapor Sensors for Electronic Nose Applications. First-principles calculations were carried out based on the density functional theory (DFT) to verify that the ultrafast recovery behavior arises from the weak van der Waals binding between NO 2 and the MoS 2 surface. The high responsivity is related to the fact that the adsorbed NO 2 can affect the electron states within the entire material, which is attributed to the very small thickness of the MoS 2 nanosheets. Interestingly, compared with other NO 2 gas sensors based on MoS 2, FLMN gas sensors exhibit high responsivity for room-temperature NO 2 detection, and NO 2 is easily desorbed from the sensor surface with an ultrafast recovery behavior, with recovery times around 2 s. 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